In 2010, he had his 25th release with Singam directed by Hari, in which he played the role of a police officer from a small village going to work in the city. The film opened to positive reviews with The Hindu noting that "Suriya shows that be it a performance-oriented role or a formulaic concoction he can deliver", while Sify.com stated "Ultimately it is Suriya who carries the film to the winning post. His passion and the way he brings an ordinary regular larger-than-life hero character alive on screen is lesson for other before also starring in K. V. Anand's Ko and Bala's Avan Ivan (2011).

His only release in 2011 that featured him in a starring role was A. R. Murugadoss's science fiction thriller 7aum Arivu. Suriya essayed dual roles in the film, as a circus artist and as the Buddhist monk named Bodhidharma, who lived in the 5th century. The film met with mixed reception, but Suriya's performance was praised. 7aum Arivu became the actor's highest grosser, and subsequently among the top grossing films of the year.